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Here you'll find links to a number of online sheet music collections that allow you to download and print complete works. These are generally in the public domain (copyright-free), but be sure to check the usage guidelines on each site beforehand!
Sheet Music Collections Online
Historic American Sheet Music Collection
Directory of large sheet music collections accessible either through a web page or an online catalog. Many of the collections include digitized reproductions of sheet music in the public domain. Hosted by the Duke University Library.
Inventions of Note: Sheet Music Collection
A small digital music collection of songs and piano music, created by MIT.
Lester S. Levy Collection of Sheet Music
A digitized collection of sheet music, available through the Special Collections at the Sheridan Libraries of the Johns Hopkins University.
Music Manuscript Online
An online collection of original manuscripts from such composers as Bach, Haydn, and Berg. Digital scans can be explored online.
Sibley Music Library: Musical Scores
An archive of sheet music put together by the Eastman School of Music (University of Rochester). Searchable by keyword, with a variety of limits (voice part, arrangement, etc.).
Templeton Digital Sheet Music Collection
Provides a searchable index of fully digitized sheet music at Mississippi State University, much of which is public domain.
VARIATIONS: Online Musical Scores
The VARIATIONS project is a prototype project, created by Indiana University, that combines musical scores, recordings, and liner notes, for a number of works (opera, orchestral, choral, solo instrument, etc.).